Natural product-based phenols as novel probes for mycobacterial and fungal carbonic anhydrases

J Med Chem. 2011 Mar 24;54(6):1682-92. doi: 10.1021/jm1013242. Epub 2011 Feb 18.

Abstract

In order to discover novel probes that may help in the investigation and control of infectious diseases through a new mechanism of action, we have evaluated a library of phenol-based natural products (NPs) for enzyme inhibition against four recently characterized pathogen β-family carbonic anhydrases (CAs). These include CAs from Mycobacterium tuberculosis, Candida albicans, and Cryptococcus neoformans as well as α-family human CA I and CA II for comparison. Many of the NPs selectively inhibited the mycobacterial and fungal β-CAs, with the two best performing compounds displaying submicromolar inhibition with a preference for fungal over human CA inhibition of more than 2 orders of magnitude. These compounds provide the first example of non-sulfonamide inhibitors that display β over α CA enzyme selectivity. Structural characterization of the library compounds in complex with human CA II revealed a novel binding mode whereby a methyl ester interacts via a water molecule with the active site zinc.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Anti-Bacterial Agents / chemical synthesis
  • Anti-Bacterial Agents / chemistry
  • Antifungal Agents / chemical synthesis
  • Antifungal Agents / chemistry
  • Biological Products / chemical synthesis
  • Biological Products / chemistry*
  • Candida albicans / enzymology*
  • Carbonic Anhydrase I / antagonists & inhibitors
  • Carbonic Anhydrase I / chemistry
  • Carbonic Anhydrase II / antagonists & inhibitors
  • Carbonic Anhydrase II / chemistry
  • Carbonic Anhydrase Inhibitors / chemical synthesis
  • Carbonic Anhydrase Inhibitors / chemistry*
  • Carbonic Anhydrases / chemistry*
  • Catalytic Domain
  • Cryptococcus neoformans / enzymology*
  • Crystallography, X-Ray
  • Humans
  • Hydrogen Bonding
  • Isoenzymes / antagonists & inhibitors
  • Isoenzymes / chemistry
  • Models, Molecular
  • Molecular Structure
  • Mycobacterium tuberculosis / enzymology*
  • Phenols / chemical synthesis
  • Phenols / chemistry*
  • Protein Binding
  • Small Molecule Libraries

Substances

  • Anti-Bacterial Agents
  • Antifungal Agents
  • Biological Products
  • Carbonic Anhydrase Inhibitors
  • Isoenzymes
  • Phenols
  • Small Molecule Libraries
  • Carbonic Anhydrase I
  • Carbonic Anhydrase II
  • Carbonic Anhydrases

Associated data

  • PDB/3NB5
  • PDB/3P4V